Let $S_{k},k = 1,2,\ldots,100$, denote the sum of the infinite geometric series whose first term is $\frac{k - 1}{k!}$ and the common ratio is $\frac{1}{k}$. Then the value of $\frac{100^{2}}{100!} + \sum_{k = 1}^{100}{2mu}\left| \left( k^{2} - 3k + 1 \right)S_{k} \right|$ is